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Na, M. X. ; Boschini, F. ; Mills, A. K. ; Michiardi, M. ; Day, R. P. ; Zwartsenberg, B. ; Levy, G. ; Zhdanovich, S. ; Kemper, A. F. ; Jones, D. J. ; et al ( , Physical Review B)null (Ed.)
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Na, M. X. ; Mills, A. K. ; Boschini, F. ; Michiardi, M. ; Nosarzewski, B. ; Day, R. P. ; Razzoli, E. ; Sheyerman, A. ; Schneider, M. ; Levy, G. ; et al ( , Science)
Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of nonthermal electrons, a material’s dominant scattering processes can be revealed. Here, we present a method for extracting the electron-phonon coupling strength in the time domain, using time- and angle-resolved photoemission spectroscopy (TR-ARPES). This method is demonstrated in graphite, where we investigate the dynamics of photoinjected electrons at the
point, detecting quantized energy-loss processes that correspond to the emission of strongly coupled optical phonons. We show that the observed characteristic time scale for spectral weight transfer mediated by phonon-scattering processes allows for the direct quantitative extraction of electron-phonon matrix elements for specific modes.